Force characteristic of the large coal particlewas investigated when it moved in a dense mediumgas–solid fluidized bed with the 100–300 μmGeldart Bmagnetite powder as fluidized medium. Weselected two groups of coal particles with the equivalent diameters of 13 and 25mmas the studying objects. The theoretical force calculation model of the large coal particle was established by force analysis. The approaches of experimental measurement and numerical simulation were combined to determine the force characteristic of the large coal particle. The results indicate that the forces vary within certain suitable ranges and present uniform fluctuations when the dense medium gas–solid fluidized bed maintains a stable fluidization state. The spectral analysis method was introduced to compare the force results of measurement and simulation. Finally, we obtain the conclusion that the theoretical force calculation results provide good agreements with the measurement and simulation results, which also validates the accuracy of the measurement results and the reliability of the simulation results for the force characteristic of the large coal particle.